1. Topic

  How to measure benzene?

2. Introduction

   

The 2nd EU Air Quality Daughter Directive deals with CO and benzene (see web link section below). Benzene is a carcinogenic compound, and the major source of benzene in air in urban areas is from gasoline, which contains a certain amount of benzene. The benzene source is partly from vehicle exhaust, partly from the handling of gasoline in pumping stations. By 1 January 2000, the maximum content of benzene in gasoline fuel in Europe was limited to 1% (http://europa.eu.int/eur-lex/pri/en/oj/dat/1998/l_350/l_35019981228en00580067.pdf), as a result of the assessment of the risk posed by benzene in air.


3. Discussion

   

The Directive describes the requirements for assessment and monitoring of benzene in air.

The position paper related to benzene (see web section below) describes the assessment of benzene in air in Europe presently, sources, risks and measurement methods.

Monitoring methods are generally based on gas chromatography, with either active (pumped) or passive (diffusive) sampling and thermal or solvent desorption prior to analysis. Automated instruments with active (pumped) sampling and thermal desorption are available, which allow for quasi continuous monitoring. Advantages and disadvantages as well as typical uncertainties of the different methods are given. Pumped sampling on tubes followed by GC analysis including calibration is recommended as basis for a reference method. A detailed reference method will be worked out by CEN.

Standard measurement methods are being developed by CEN (under approval, as of December 2004):

· prEN 14662-1: Pumped sampling followed by thermal desorption and gas chromatography;

· prEN 14662-2: Pumped sampling followed by solvent desorption and gas chromatography;

· prEN14662-3: Automated pumped sampling with in situ gas chromatography;

· prEN 14662-4: Diffusive sampling followed by thermal desorption and gas chromatography;

· p2EN 14662-5: Diffusive sampling followed by solvent desorption and gas chromatography.

Brief description of methods:

On-line gas chromatographs are available either as BTX-monitors (Benzene, Toluene, Xylene), measuring benzene, toluene, ethyl benzene and xylenes or more capable of measuring C2-C10 hydrocarbons. These instruments are based on the same principle.

Canister sampling is performed in two ways either as grab sampling or as pumped sampling. The grab sampling is carried out by opening an evacuated canister, which instantaneously fills the canister with ambient air up to ambient pressure. Alternatively, air can be pumped into the canister over time in order to obtain an integrative sample. The canisters are then brought to the laboratory where they are analysed by gas chromatography (GC).

Pumped sorbent tube sampling is performed by pumping ambient air through a tube filled with a sorbing material. The trapped benzene is removed by solvent extraction or thermal desorption followed by GC analysis.

Diffusive sampling of benzene is performed by placing benzene adsorbent in a glass or metal tube. The sampler collects benzene by diffusion (following Fick's first law) due to the gradient established between ambient air and the adsorbing material. Benzene is removed from the sampler by solvent extraction or thermal desorption and in both cases benzene is analysed by GC.

DOAS (Differential Optical Absorption Spectroscopy) is an open path.

Optical measuring technique applicable for a number of gases which includes benzene. This method has so far not been through a standardization procedure.

Quality control of monitoring data

Annex VIII of the 1st and 3rd Daughter Directives (see web links below) specify the required accuracy of measurement data, as well as the minimum data capture (parts of the year the measurement data must be available from a monitoring station). These requirements are laid down as a guide to what quality-control and –assurance (QA/QC) programmes that monitoring network operators need to follow to comply with the quality objectives. QA/QC procedures are dealt with in the Topic How to secure the quality of the monitoring data? Quality assurance (QA) and Quality Control (QC) systems and procedures..


4. Recommendation / Conclusion

   

· The proper monitoring of air pollutants like the ones considered in this topic description requires knowledge of and experience with the methods to be used, of considerations for monitoring network design, as well as of needed additional resources, such as needed laboratory support, and of quality control and assurance procedures.

· This knowledge and experience must be embedded within the local or other authority or institution responsible for the monitoring.


5. Examples / Further Reading

   

How to monitor Benzene Emissions of VOCs from petrol stations - a review; 1995 to 2003.

The MacBeth Project: Passive Samplers Measurements of Benzene Levels in the City of Padua (I)


6. Additional Documents / Web Links

   

· 2nd Daughter Directive on CO and benzene: http://www.europa.eu.int/cgi-bin/eur-lex/udl.pl?COLLECTION=lif&SERVICE=eurlex&REQUEST=Seek-Deliver&GUILANGUAGE=en&LANGUAGE=en&DOCID=300L0069

· Position paper on benzene: http://europa.eu.int/comm/environment/air/pdf/pp_benzene.pdf

· Technical report No 11, Guidance report on preliminary assessment under EC air quality directives: http://reports.eea.eu.int/TEC11a/en/tab_content_RLR

· Technical guidance documents: http://www.defra.gov.uk/environment/airquality/laqm/guidance/pdf/laqm-tg03.pdf and http://www.umweltbundesamt.de/index-e.htm

· Directive on quality of motor vehicle fuel, limiting the benzene contents of gasoline: http://europa.eu.int/eur-lex/pri/en/oj/dat/1998/l_350/l_35019981228en00580067.pdf


Last Updated


 

21st January 2005

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